Can one use H NMR assignments to make C NMR assignments?

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JoeyBobBillie
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Can one use H NMR assignments to make C NMR assignments?

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For instance, with a more complex molecule where COSY is used to make H NMR assignments. Will the lowest H NMR signal be attached to the carbon with the lowest C NMR signal, then the second lowest matched with the second lowest ect.?
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